The largest crystals of Natrolite, as single floaters, were found in the Khibiny Massif, Kola Peninsula, Russia. These crystals were very scarce and are hard to come across; only a very limited supply of them was ever released from the find. In Australia, rounded spiky puffs come from Cape Grim, Tasmania. The Indian basalt deposits, known for their spectacular zeolite minerals, are surprisingly scarce in Natrolite. Although the related mineral Scolecite is fairly abundant in the state of Maharashtra, India, Natrolite has been found only sparingly, in the cities of Pune (Poona), Mumbai, and Nasik, mostly as elongated brittle sprays.
In Europe, pink and brownish globular formations of Natrolite have come from the Ústí Region, Bohemia, Czech Republic. White slender crystal groups have come from Puy de Marmant, Puy de Dôme, France; and white and light pink needle sprays from Piz Sella, Bolzano Province, Italy.
In the U.S., the state of New Jersey is the most prolific producer of Natrolite, with several important deposits. Acicular groupings are abundant at the Upper New St. Quarry, Paterson, Passaic Co. Nearby Prospect Park, Passaic Co. has also produced nice acicular Natrolite, sometimes with pinkish tones. Very large crystals up to 10 cm., sometimes water-clear, have come from the Chimney Rock Quarry, Bound Brook, Somerset Co., New Jersey. Snow-white crystal groupings and acicular balls in very aesthetic formation were once prevalent at the Millington Quarry, Somerset Co., New Jersey.
Natrolite is a white massive matrix of micro-crystals for the rare minerals Benitoite and Neptunite at the Dallas Mine, San Benito Co., California. Natrolite has also occurred there as a single gemmy elongated crystals in occasional finds. Hemispherical Natrolite balls are well-known from the Horseshoe Dam area, Maricopa Co., Arizona. In Canada, water-clear, flawless crystals were found at Mont Saint Hilaire, Quebec, as well in white crystals and groups associated with Serandite. In Nova Scotia, Natrolite can be found at Wasson's Bluff in Parrsboro, and at the Five Islands area.